ADVANCED MATERIALS先进材料
ADVANCED MATERIALS(英文缩写 ADV MATER),ISSN 0935-9648,eISSN 1521-4095,中文译名:先进材料 是一本学术期刊。本页汇总该期刊的最新影响因子、分区信息以及最新收录于 PubMed 的文献,帮助您快速了解期刊全貌。
发文量统计区间：2025-09-01 至 2026-08-31，按本站收录文献的发表日期统计。
期刊介绍
历年影响因子趋势
| JCR 数据年份 | 影响因子 | JCR 分区 |
|---|---|---|
| 2021 | 32.086 | Q1 |
| 2022 | 29.400 | Q1 |
| 2023 | 27.400 | Q1 |
| 2024 | 26.800 | Q1 |
| 2025 | 29.100 | Q1 |
ADVANCED MATERIALS 最新收录文献
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1. Bone-Targeted Engineered Exosomes Delivering Betaine Alleviate Osteoporosis via Autophagy-Driven Osteogenesis.
PMID:日期:2026-09-27Dysregulated bone remodeling, attenuated endogenous osteogenic capacity, and the lack of bone-targeting capability in therapeutics constitute the core challenges in current clinical interventions for osteoporosis. In this study, a hybrid nanodelivery system integrating betaine-loaded metal-organic frameworks with engineered exosomes (BZ@Exos) is constructed to restore bone metabolic homeostasis and improve bone microstructure. The engineered exosomes co-overexpressing CXCR4 and CD47 proteins on the surface exhibit high bone tissue targeting efficiency and evade clearance by the mononuclear phagocyte system, while ZIF-8 enables stable encapsulation of betaine. Internalized betaine promotes nuclear translocation of TFEB via targeted binding to the 14-3-3 protein, enhances autophagic flux in senescent bone marrow mesenchymal stem cells (BMSCs), and thereby facilitates their osteogenic differentiation. In parallel, BZ@Exos significantly inhibits osteoclast-mediated bone resorption and restores bone metabolic homeostasis. In vivo assays demonstrate that intravenously administered BZ@Exos successfully reverses bone loss and alleviates senescence-related phenotypes in ovariectomized rat models of osteoporosis. This novel therapeutic system with integrated functions of bone homeostasis remodeling, regenerative potential restoration, and precise targeting provides a new perspective for osteoporosis treatment.
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2. Fiber-Format Flexible Linear Electrostatic Motors.
PMID:日期:2026-09-27Linear motion is fundamental to robotics, yet existing solutions are either rigid electromagnetic motors or contractile artificial muscles with limited stroke and trade-offs in force versus displacement. We report a sliding motor in a thin fiber format: a flexible, electrostatic linear actuator with a stroke limited only by fiber length. Comprising two coaxial fibers with helically wound electrodes, this "FiberMotor" generates bidirectional, fast, stepping motion with stroke-independent force and inherent back-drivability, a key feature for safe and transparent human-robot interaction. By eliminating permanent magnets and Joule heating, it offers a compact alternative to traditional motors. Modular bundling allows scaling to higher forces. Supported by an analytical model, this silent, lightweight technology can enable large-scale integration into textiles, providing a promising building block toward future soft exosuits and wearable assistive devices.
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3. Percolation-Driven β-Relaxation Enables Resonant Acceleration of Crystallization in Amorphous Phase-Change Materials.
PMID:日期:2026-09-27Amorphous phase-change materials enable fast and reversible switching in optical and electronic devices, yet crystallization kinetics are still controlled primarily through empirical thermal protocols. Here we identify a microscopic picture governing crystallization in the prototypical phase-change material GeSbTe, in which crystallization pathways are organized by the percolation of mobile atomic networks associated with β-relaxation. We show that this percolation transition distinguishes the dominance of diffusion-driven and diffusionless nucleation and growth during crystallization processes. We further demonstrate that frequency-selected ultrasonic excitation, applied in conjunction with heating, accelerates crystallization by enhancing percolation-mediated atomic dynamics. This acceleration is maximized near the β-relaxation frequency, consistent with resonant excitation of mobile atoms. Our results establish a direct link between glassy relaxation, atomic-scale percolation, and crystallization, and introduce a new route to modulating phase-change kinetics through targeted excitation of fundamental glassy dynamics.
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4. Precursor-Level Molecular Coupling Enables High-Fill-Factor Wide-Bandgap Perovskite Solar Cells and 29.63% All-Perovskite Tandems.
PMID:日期:2026-09-27Wide-bandgap (WBG) perovskites with a ∼1.78 eV bandgap are essential for monolithic all-perovskite tandem cells, yet their efficiency and stability are limited by complex precursor chemistry, uncontrolled crystallization, defect formation, and photoinduced halide segregation. Here, we report 4-(3-Carbamimidoylguanidino)benzoic acid hydrochloride (CGBA) as a precursor-level regulator for Cs/formamidinium (CsFA)-based Br-rich WBG perovskites. Through dynamic associations with lead-halide species and organic cations, CGBA modifies the local precursor environment and alters the stage-dependent film-formation behavior during spin coating and annealing. This regulation moderates crystallization, promotes texture development, reduces trap-mediated nonradiative recombination, and suppresses photoinduced halide segregation. Consequently, the optimized 1.78 eV single-junction device achieves a power conversion efficiency (PCE) of 21.43% and a fill factor (FF) of 85.89%, placing it among the highest reported FF values for 1.75-1.79 eV single-junction WBG perovskite solar cells. The strategy is also transferable across multiple compositions and conditions, yielding efficiencies of 27.32% (1.53 eV), 23.91% (1.68 eV), 18.75% (1.85 eV), and 26.08% (1.58 eV, antisolvent-free). Unencapsulated target devices retain 93% of their initial efficiency after 4500 h in N. When integrated into a monolithic all-perovskite tandem, the CGBA-optimized WBG subcell enables a laboratory-measured PCE of 29.63%. This work establishes precursor-level regulation as a transferable strategy for efficient and stable WBG perovskites and all-perovskite tandems.
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5. Over 20% Efficiency in As-Cast Organic Solar Cells Enabled by Flory-Huggins Parameter Engineering.
PMID:日期:2026-09-27The realization of high-efficiency as-cast organic solar cells (OSCs) represents a key step toward simplified processing and scalable fabrication for commercialization. However, achieving high-performance as-cast devices remains challenging because it demands delicate balance between donor-acceptor self-aggregation and miscibility. Herein, we fabricate as-cast OSCs through Flory-Huggins parameter (χ) engineering that precisely regulates donor-acceptor miscibility during solution casting. The chloroform-carbon disulfide (CF:CS) mixed solvent, with tailored solubility and evaporation kinetics, dynamically modulates χ to form an optimized bulk heterojunction featuring desirable phase separation and a well-balanced fibrillar network. This design affords efficient exciton dissociation, facilitated charge transport, and suppressed recombination in the blend. Consequently, as-cast D18:L8-BO device processed with the CF:CS solvent system attained a PCE of 20.11% (certified as 19.69%) alongside enhanced photostability, representing the highest efficiency reported for as-cast devices. Besides, high PCEs of 18.89% and 15.12% are achieved in thick-film (300 nm) and large-area (20.17 cm) as-cast devices. Moreover, a quantitative correlation between PCE and the interaction parameter χ is established, providing a quantitative guide for narrowing the miscibility window and identifying the optimal composition. These findings validate the efficacy of χ-parameter-mediated miscibility engineering in regulating blend phase behavior and provide a framework for advancing efficient as-cast OSCs.
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6. Locally Water-Rich Interfacial Microenvironment Enables Self-Powered High-Current Ammonia Electrosynthesis.
PMID:日期:2026-09-27Electrochemical nitrate-to-ammonia conversion holds great promise for sustainable nitrogen fixation, yet its industrial‑level current density operation is limited by cathodic active hydrogen (*H) supply shortage and high energy consumption caused by anodic oxygen evolution reaction (OER). Here, we develop a bifunctional CoP electrocatalyst with engineered phosphorus vacancies that generate atomic-scale electric fields to enrich interfacial water molecules via enhanced hydrogen-bonding interactions, alleviating local water scarcity caused by double-layer compression under high nitrate concentrations and promoting *H generation for nitrate reduction reaction (NORR). Meanwhile, we replace OER with the thermodynamically favorable hydrazine oxidation reaction (HzOR), and the electrocatalyst promotes *OH adsorption to facilitate hydrazine dehydrogenation in HzOR. The resulting NORR||HzOR electrolyzer delivers an ammonia yield of 49.64 mg h cm at 500 mA cm with a cell voltage of 0.962 V, and enables self-powered ammonia production at 0.769 g L h without external energy input. This work reveals atomic-scale electric field engineering as an effective strategy to modulate interfacial microenvironment for high-performance, low-energy ammonia electrosynthesis.
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7. Bare-Die Antiferromagnetic Computing.
PMID:日期:2026-09-27Semiconductor electronic devices are increasingly constrained by fundamental quantum tunneling effects and charge-based mechanisms, which severely limit further miniaturization, write-speed scaling, and environmental robustness of silicon-based technologies. These limitations are particularly prohibitive for deep-space exploration, where extreme temperatures, ultra-strong magnetic fields, and intense radiation rapidly incapacitate conventional electronics without massive shielding. Here, we present an intrinsically resilient, strain-mediated antiferromagnetic MnIr/PMN-PT edge processor that operates reliably as a bare die under temperatures up to 500 K, magnetic fields of 55 T, and radiation doses of 1.5 Mrad. By exploiting an Input-Modulated In Situ Self-Refreshing Encoding mechanism, the device performs nonlinear feature extraction and classification directly from raw analog signals, enabling an analog computing architecture that requires no time-frequency transformation. This architecture achieves 99.8% accuracy in speech recognition without digital preprocessing and 100% accuracy in astronaut visual object recognition. Furthermore, an all-hardware integrated drone vision system demonstrates real-time in situ command execution and autonomous navigation, delivering a terahertz-level response frequency and an ultra-low energy consumption of approximately 0.2 fJ per operation. This work expands the functional scope of antiferromagnetic devices beyond memory and logic, establishing them as a promising materials platform for energy-efficient physical computing and autonomous intelligence in extreme environments.
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8. Atmosphere-Controlled Valence Engineering of Eu in Aluminate Crystals Enabling High-Performance Temperature Sensing and Flexible X-Ray Imaging.
PMID:日期:2026-09-27Developing scintillators that simultaneously deliver high light yield, radiation stability, flexibility, and environmental sustainability remains a long-standing challenge, while optical thermometry is further limited by narrow working ranges and insufficient sensitivity. Here, we propose a buried-carbon reduction concept that enables precise regulation of Eu valence states through controlled carbon burial depth from a single precursor, thereby unlocking multifunctionality within one material system. By such strategy, fully reduced SrMgAlO:Eu is utilized in x-ray detection and imaging. High-energy irradiation activates defect-mediated electron release, substantially increasing the effective concentration of luminescent centers. Remarkably, its radioluminescence intensity retains 117.5% after over 150 on-off irradiation cycles, showing a long-term working light yield of up to 55917 ± 573 photons MeV, together with excellent linear dose response and a low detection limit. Flexible scintillator films achieve a spatial resolution of 11.7 lp mm(at 20% MTF). These characteristic makes the material with low cost, flexibility, environmental protection, chemically stable, and excellent radiation resistance. Moreover, partially reduced SrMgAlO:Eu/Eu exhibits rare multimodal synergistic optical thermometry performance in the high-temperature region owing to distinct thermal quenching behaviors. In the temperature range of 550-625 K, the FIR-based S and S reach 0.226 K and 0.97 %K, respectively; the FWHM-based thermometric mode achieves a maximum sensitivity of 0.238 nm/K, while also enabling visual discrimination of the temperature. This work establishes a versatile concept for designing advanced optical materials for radiation detection and temperature sensing.
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9. Targeting FAK-YAP Signaling Axis Inhibits Tumor Stemness and Overcomes Tumor Resistance to Cuproptosis.
PMID:日期:2026-09-26Cuproptosis has recently been identified as a novel metabolic cell death pathway that holds great promise for cancer therapy. However, cuproptosis resistance developed by tumor cells severely impairs its anticancer efficacy. Here, our study uncovers that the FAK-YAP signaling axis in tumor cells plays important roles in the development of cuproptosis resistance and the promotion of tumor stemness. To therapeutically target this signaling axis, a CRISPR-cuproptosis synergistic nanoplatform (CPLNP@HA) is elaborately designed for targeted co-delivery of a Ptk2 (encoding FAK) CRISPR-Cas9 knockout plasmid to block FAK-YAP signaling axis and Cu-elesclomol (Cu-ES, a cuproptosis inducer) into tumor cells. Mechanistically, CPLNP@HA efficiently silences FAK expression, which subsequently blocks the cuproptosis-induced activation of the FAK-YAP signaling cascade. This intervention not only sustains intracellular copper accumulation to reinforce cuproptosis but also reduces tumor stemness, thereby significantly potentiating the therapeutic outcomes of cuproptosis and activating tumoricidal immunity as evidenced by transcriptomic analysis. In combination with immune checkpoint blockade therapy, CPLNP@HA markedly inhibits tumor development upon rechallenge after surgical resection. Our work establishes FAK-YAP signaling axis as a new therapeutic target to overcome cuproptosis resistance and inhibit tumor stemness, providing a promising combinatorial paradigm to sensitize tumor to cuproptosis and immunotherapy.
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10. Inverse Design of Nanoparticulate Materials.
PMID:日期:2026-09-25The unique size- and shape-dependent properties of nanomaterials offer a rich parameter space for tailoring functionalities and applications. Recently, inverse design of such nanoparticulate systems has provided a paradigm shift from empirical trial-and-error approaches toward predictive, model-driven design strategies to achieve desired functionalities. This perspective presents a practical framework for applying inverse design to nanoparticulate materials. We distinguish between two general modeling strategies: knowledge-based design, grounded in a detailed understanding of the underlying physics and chemistry, and data-based design, based on experimental or simulated input-output datasets. Hybrid models bridge these two strategies. Each strategy is further structured into three levels of optimization: (i) process optimization via process functions connecting synthetic parameters with resulting particle properties; (ii) structure optimization via property functions connecting particle properties with macroscopic properties; and (iii) full inverse design via combined property-process relationships. In a tutorial style, we introduce practical steps for model development, calibration, and implementation and discuss design rules to guide the choice of modeling strategy. This perspective thus aims to facilitate the broad adoption of inverse design for nanoparticulate systems, laying the foundation for the development of rigorously optimized, application-specific materials with ideal properties tailored to a given application.